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  • 1
    Online Resource
    Online Resource
    AIP Publishing ; 2006
    In:  Journal of Applied Physics Vol. 99, No. 8 ( 2006-04-15)
    In: Journal of Applied Physics, AIP Publishing, Vol. 99, No. 8 ( 2006-04-15)
    Abstract: Rare-earth atoms play an important role in determining the magnetocrystalline anisotropy in 4f-3d intermetallic compounds. Recently we reported on the synthesis and magnetic properties of Gd-substituted Mn-Zn ferrite nanoparticles as potentially suitable for magnetic fluid hyperthermia (MFH). In MFH the specific power absorption rate is related to the lossy magnetocrystalline anisotropic properties of the magnetic fluids. In this paper we report the role of Ho substitution in magnetite nanoparticles, which is found to enhance the KV product arising from the large anisotropy of Ho3+ moments. The zero-field-cooled magnetization data is then simulated by assuming noninteracting magnetic particles with uniaxial anisotropy and lognormal particle size distribution. The fit parameters give the values of particle diameter (D) 9 nm, standard deviation 0.3 in ln(D), and the anisotropy constant K to be 3.5×104J∕m3. The value of K thus obtained is an order of magnitude larger than the value known for the undoped for magnetite (104J∕m3).
    Type of Medium: Online Resource
    ISSN: 0021-8979 , 1089-7550
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2006
    detail.hit.zdb_id: 220641-9
    detail.hit.zdb_id: 3112-4
    detail.hit.zdb_id: 1476463-5
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  • 2
    Online Resource
    Online Resource
    AIP Publishing ; 2000
    In:  Journal of Applied Physics Vol. 88, No. 5 ( 2000-09-01), p. 2799-2804
    In: Journal of Applied Physics, AIP Publishing, Vol. 88, No. 5 ( 2000-09-01), p. 2799-2804
    Abstract: Electron spin resonance spectra of a temperature sensitive magnetic fluid involving polydispersed Mn0.5Zn0.5Fe2O4 ferrite particles are scanned from 200 to 400 K. For such a polydispersed system, the deconvolutions of the spectra suggest coexistence of two different resonance modes: (i) a broad line due to ferrimagnetic resonance and (ii) a sharp line at g=2 due to intrinsic superparamagnetic phase. From the intensity variation of the line at g=2, it is found that the contribution due to the superparamagnetic phase increases with temperature. A study of peak-to-peak linewidth variation with temperature indicates that the weakening of the magnetic moment is responsible for the observed reduction in the linewidth.
    Type of Medium: Online Resource
    ISSN: 0021-8979 , 1089-7550
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2000
    detail.hit.zdb_id: 220641-9
    detail.hit.zdb_id: 3112-4
    detail.hit.zdb_id: 1476463-5
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  • 3
    In: AIP Advances, AIP Publishing, Vol. 5, No. 4 ( 2015-04-01)
    Abstract: Structural, electrical and magnetic properties of magneto-electric composite ceramics viz., 0.9 BaTi0.95Sn0.05O3 (BTSO)- 0.1 Ni0.8Zn0.2Fe2O4 (NZFO) prepared with microwave assisted radiant hybrid sintering (MARH) are reported. Phase purity and isovalent substitution of Ti4+ by Sn4+ of the samples is confirmed from x-ray diffraction and 119Sn Mossbauer measurements respectively. Significant suppression of leakage current and improvement of ferroelectricity is observed for the composites prepared with MARH. The observed results are explained in terms of uniform dispersion of ferrite (NZFO) phase in the ferroelectric (BTSO) matrix as evidenced from back-scattered scanning electron micrographs.
    Type of Medium: Online Resource
    ISSN: 2158-3226
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2015
    detail.hit.zdb_id: 2583909-3
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  • 4
    Online Resource
    Online Resource
    AIP Publishing ; 2013
    In:  Journal of Applied Physics Vol. 113, No. 21 ( 2013-06-07)
    In: Journal of Applied Physics, AIP Publishing, Vol. 113, No. 21 ( 2013-06-07)
    Abstract: Epitaxial BiFeO3 (BFO) films were deposited using pulsed laser deposition method. The prepared films were characterized using x-ray diffraction, x-ray reflectivity, ferroelectric loop tracer, and leakage current measurements before and after oxygen plasma treatment. The leakage current of the films, a crucial parameter in device applications, is observed to be reduced by two orders of magnitude with oxygen plasma treatment at room temperature. P-E hysteresis loops were observed in oxygen plasma treated BFO films. The observed results indicate the usefulness of oxygen radio frequency plasma treatment (RF 13.56 MHz), which is an effective and low temperature processing technique, in such lossy ferroelectric thin films.
    Type of Medium: Online Resource
    ISSN: 0021-8979 , 1089-7550
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2013
    detail.hit.zdb_id: 220641-9
    detail.hit.zdb_id: 3112-4
    detail.hit.zdb_id: 1476463-5
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  • 5
    Online Resource
    Online Resource
    AIP Publishing ; 2013
    In:  Journal of Applied Physics Vol. 114, No. 21 ( 2013-12-07)
    In: Journal of Applied Physics, AIP Publishing, Vol. 114, No. 21 ( 2013-12-07)
    Abstract: Magnetorheological (MR) properties are experimentally investigated for bi-dispersion suspension of plate-like iron magnetic particles dispersed in carrier liquid to see the influence of small size particle on large size MR fluid. As a first step, structural, magnetic, and morphology of two different micron size magnetic particles are described in details. The three different weight fractions of MR fluid samples are then prepared, followed by measuring their magneto-viscous and visco-elastic properties. In the steady-state shear, the Bingham yield stress obtained by extrapolating the shear stress to the zero shear rate increases by augmenting the weight fraction of small micron size magnetic particles and the strength of magnetic field. In the oscillatory strain sweep test at an angular frequency of 10 rad s−1, a transition from visco-elastic solid to visco-elastic liquid is observed and a strong chain formation is proposed to explain the mechanism for transition. The storage modulus also increases with increasing weight fraction. From the frequency sweep test, the storage modulus is seen as independent of frequency, but depends on the magnetic field strength and weight fraction. The magneto-viscous sweep test indicates that both shear modulus and complex viscosity are independent with weight fraction at a high magnetic field. This experimental study reveals some very important physical parameters, rheological properties, and storage modulus of the plate-like iron particles based on MR fluid. The formation of less compact because of the anisotropy in iron particle creates weak sedimentation and good redispersibility of MR fluid. The results presented in this work are the key factors for devising how mechanical applications operated under static and dynamic conditions.
    Type of Medium: Online Resource
    ISSN: 0021-8979 , 1089-7550
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2013
    detail.hit.zdb_id: 220641-9
    detail.hit.zdb_id: 3112-4
    detail.hit.zdb_id: 1476463-5
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  • 6
    In: Physics of Plasmas, AIP Publishing, Vol. 26, No. 1 ( 2019-01-01)
    Abstract: We report angular and spectral distribution of fast electrons in the interaction of a high intensity laser pulse (30 fs, I∼1019 W/cm2) with uncoated transparent mylar foil (thickness: 8 μm). The effect of thin Al coating (50 nm) on either the front or rear surface of the mylar foil on fast electron generation was also investigated. An electron flux enhancement of ∼1.8× (from ∼45 pC to ∼80 pC) and an increase in the maximum electron energy from ∼ 400 keV to ∼ 800 keV were observed in the case of front coated foil compared to the uncoated one. In the case of rear coated foil, an enhancement of ∼1.4× in the electron flux with no change in maximum electron energy was observed compared to the uncoated foil. The observations are understood in terms of possible different preplasma conditions for various target configurations used, which is also supported by 1D hydrodynamic simulation carried out for the present experimental conditions. The observed enhancement in electron flux and temperature is also supported by 2D Particle in Cell (PIC) simulation.
    Type of Medium: Online Resource
    ISSN: 1070-664X , 1089-7674
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2019
    detail.hit.zdb_id: 1472746-8
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  • 7
    In: Physics of Plasmas, AIP Publishing, Vol. 26, No. 4 ( 2019-04-01)
    Abstract: We report a study on the generation of relativistic fast electrons during the interaction of an ultrashort (45 fs) laser pulse with a variety of targets (Al, Cu, Mo, Si, polyvinyl chloride, and Perspex), at a nearly grazing angle of incidence (∼70°) at an intensity of ∼1.2 × 1018 W/cm2. The fast electron emission direction was found to be dependent on the laser pulse amplified spontaneous emission (ASE) contrast, its extent, and laser pulse duration. For a 45 fs laser pulse and an ASE extent of 1 ns, the electron emission direction changes from a nearly target surface (∼7° ± 2°, divergence: ∼30°) to a specular direction (∼20° ± 2°, divergence: ∼20°) when the contrast was decreased from ∼10−7 to ∼10−6. It further shifts toward target normal with an increase in the ASE duration from 1 ns to 5 ns. For an ASE contrast of ∼10−7 and ∼10−6 with a 1 ns duration, preplasma density scale lengths of ∼30 μm and ∼45 μm were estimated, respectively, from the HELIOS hydrodynamic code. For a longer ASE duration in the range of 1–5 ns, the density scale length was in the range of ∼45–140 μm. Further, for a 45 fs pulse and a 1 ns ASE level, the electron beam charge was found to be higher in the case of Mo (∼52 pC) and Si (∼122 pC) targets compared to the other targets (∼23–34 pC). A further increase in the charge of the electron beam of ∼1.45× (∼75 pC) and ∼2.7× (∼141 pC) was also observed with Mo for a longer pulse duration of ∼170 fs (ASE 1 ns) and a larger ASE duration of 5 ns at (45 fs pulse), respectively. The electron beam properties were found to be independent of laser polarization (p, s, and circular) except a slightly higher charge (∼1.5×) was observed in the case of p-polarized laser light. The fast electron spectrum showed a maximum energy of 1 MeV with electron temperatures of ∼390 keV and ∼320 keV for the target surface and specular direction, respectively. Electron acceleration and their emission are explained in terms of applicable mechanisms in preformed plasma on the target surface considering the role of surface fields which is also established by the 2D particle in cell simulation.
    Type of Medium: Online Resource
    ISSN: 1070-664X , 1089-7674
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2019
    detail.hit.zdb_id: 1472746-8
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  • 8
    Online Resource
    Online Resource
    AIP Publishing ; 2018
    In:  Applied Physics Letters Vol. 112, No. 26 ( 2018-06-25)
    In: Applied Physics Letters, AIP Publishing, Vol. 112, No. 26 ( 2018-06-25)
    Abstract: We report the results of detailed investigations of magnetization, heat-capacity, dielectric, pyrocurrent, and magneto(di)electric measurements on Tb2BaCoO5, belonging to a hitherto unexplored spin-chain cobaltate family, R2BaCoO5 (R = Rare-earths). The magnetic measurements reveal that this compound exhibits an antiferromagnetic transition at (TN=) 18.8 K and there is a spin reorientation beyond 40 kOe below TN. Dielectric and pyrocurrent data measured as a function of temperature and magnetic field establish that this compound is a “type-II” multiferroic material. The most fascinating finding which we would like to emphasize is that the observed value of the magneto-dielectric effect beyond the metamagnetic transition field is the largest (close to 55%, below 10 K, for H = ∼100 kOe) ever reported for polycrystals of a compound in the bulk form, thereby offering a hope to find a single-phase polycrystalline compound at room temperature to enable ease of applications.
    Type of Medium: Online Resource
    ISSN: 0003-6951 , 1077-3118
    RVK:
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2018
    detail.hit.zdb_id: 211245-0
    detail.hit.zdb_id: 1469436-0
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  • 9
    In: The Journal of Chemical Physics, AIP Publishing, Vol. 158, No. 20 ( 2023-05-28)
    Abstract: A low-frequency dielectric response of a ferrofluid based on transformer oil and MnZn ferrite nanoparticles is investigated in a gradient magnetic field. Four ferrofluid samples of various nanoparticle concentrations were introduced into planar micro-capacitors located over a magnetized tip. The dielectric spectra were measured in the frequency range from 0.1 Hz to 200 kHz and in the local magnetic field up to 100 mT. The spectra exhibit a dielectric relaxation ascribed to nanoparticle interfacial polarization. The low-frequency spectrum of each ferrofluid decreases upon application of the magnetic field up to 20 mT. The decrease in dielectric permittivity is caused by a magnetic force acting on larger nanoparticles in the gradient magnetic field. It is assumed that the interfaces of the concentrated nanoparticles in the gradient field do not contribute to the effective dielectric response. This reduces the effective relaxation time and shifts the relaxation toward higher frequencies. The dielectric spectra are well described by a relaxation fit function consisting of one Havriliak–Negami and a conductivity term. The fitting confirms that the only effect of the gradient magnetic field on the dielectric spectra is the shift of the dielectric relaxation and the decrease of the amplitude in the imaginary permittivity. This behavior is evident from a master plot, where all dielectric relaxations are superimposed on a single line. The knowledge of the presented behavior of the ferrofluid may be valuable when applying a ferrofluid to sharply magnetized parts of various electrical equipment (wires, tips, screws, nails, edges) as a liquid dielectric medium.
    Type of Medium: Online Resource
    ISSN: 0021-9606 , 1089-7690
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2023
    detail.hit.zdb_id: 3113-6
    detail.hit.zdb_id: 1473050-9
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  • 10
    Online Resource
    Online Resource
    AIP Publishing ; 2007
    In:  Applied Physics Letters Vol. 91, No. 2 ( 2007-07-09)
    In: Applied Physics Letters, AIP Publishing, Vol. 91, No. 2 ( 2007-07-09)
    Abstract: The authors use first-principles pseudopotential-based density functional theory calculations of phonon dispersions to determine the size dependence of thermal properties of armchair single wall carbon nanotubes (SWCNTs), such as their negative thermal expansion and specific heat. While the specific heat is found to depend rather weakly on the diameter of SWCNTs, their negative thermal expansion behavior determined within a quasiharmonic approximation (QHA) exhibits a relatively strong dependence on the diameter. They identify the low energy vibrational modes that are responsible for the negative thermal expansion.
    Type of Medium: Online Resource
    ISSN: 0003-6951 , 1077-3118
    RVK:
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2007
    detail.hit.zdb_id: 211245-0
    detail.hit.zdb_id: 1469436-0
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