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  • 1
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 19, No. 6 ( 2019-03-20), p. 3515-3556
    Abstract: Abstract. The Copernicus Atmosphere Monitoring Service (CAMS) reanalysis is the latest global reanalysis dataset of atmospheric composition produced by the European Centre for Medium-Range Weather Forecasts (ECMWF), consisting of three-dimensional time-consistent atmospheric composition fields, including aerosols and chemical species. The dataset currently covers the period 2003–2016 and will be extended in the future by adding 1 year each year. A reanalysis for greenhouse gases is being produced separately. The CAMS reanalysis builds on the experience gained during the production of the earlier Monitoring Atmospheric Composition and Climate (MACC) reanalysis and CAMS interim reanalysis. Satellite retrievals of total column CO; tropospheric column NO2; aerosol optical depth (AOD); and total column, partial column and profile ozone retrievals were assimilated for the CAMS reanalysis with ECMWF's Integrated Forecasting System. The new reanalysis has an increased horizontal resolution of about 80 km and provides more chemical species at a better temporal resolution (3-hourly analysis fields, 3-hourly forecast fields and hourly surface forecast fields) than the previously produced CAMS interim reanalysis. The CAMS reanalysis has smaller biases compared with most of the independent ozone, carbon monoxide, nitrogen dioxide and aerosol optical depth observations used for validation in this paper than the previous two reanalyses and is much improved and more consistent in time, especially compared to the MACC reanalysis. The CAMS reanalysis is a dataset that can be used to compute climatologies, study trends, evaluate models, benchmark other reanalyses or serve as boundary conditions for regional models for past periods.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2019
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 2
    In: Quarterly Journal of the Royal Meteorological Society, Wiley, Vol. 136, No. 651 ( 2010-07), p. 1457-1472
    Abstract: During the 2006 African Monsoon Multidisciplinary Analysis (AMMA) field experiment, an unprecedented number of soundings were performed in West Africa. However, due to technical problems many of these soundings did not reach the Global Telecommunication System and therefore they could not be included in the operational numerical weather prediction (NWP) analyses. This issue, together with the realization that there was a significant bias in the radiosonde humidity, led to the conclusion that a re‐analysis effort was necessary. This re‐analysis was performed at the European Centre for Medium‐Range Weather Forecasts (ECMWF) spanning the wet monsoon season of 2006 from May–September. The key features of the ECMWF AMMA re‐analysis are presented, including the use of a newer model version with improved physics, all the AMMA radiosonde data available from the AMMA database and a new radiosonde humidity bias‐correction scheme. Data‐impact experiments show that there is a benefit from these observations, but also highlight large model physics biases over the Sahel that cause a short‐lived impact of the observations on the model forecast. The AMMA re‐analysis is compared with independent observations to investigate the biases in the different parts of the physics. In the framework of the AMMA project, a hybrid dataset was developed to provide a best estimate of the different terms of the water cycle. This hybrid dataset is used to evaluate the improvement achieved from the use of extra AMMA observations and of a radiosonde humidity bias‐correction scheme in the water cycle of the West African monsoon. Finally, future model developments that offer promising improvements in the water cycle are discussed. Copyright © 2010 Royal Meteorological Society
    Type of Medium: Online Resource
    ISSN: 0035-9009 , 1477-870X
    URL: Issue
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    Language: English
    Publisher: Wiley
    Publication Date: 2010
    detail.hit.zdb_id: 3142-2
    detail.hit.zdb_id: 2089168-4
    SSG: 14
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  • 3
    In: Environmental Research Letters, IOP Publishing, Vol. 17, No. 1 ( 2022-01-01), p. 014015-
    Abstract: The Paris Agreement establishes a transparency framework for anthropogenic carbon dioxide (CO 2 ) emissions. It’s core component are inventory-based national greenhouse gas emission reports, which are complemented by independent estimates derived from atmospheric CO 2 measurements combined with inverse modelling. It is, however, not known whether such a Monitoring and Verification Support (MVS) capacity is capable of constraining estimates of fossil-fuel emissions to an extent that is sufficient to provide valuable additional information. The CO 2 Monitoring Mission (CO2M), planned as a constellation of satellites measuring column-integrated atmospheric CO 2 concentration (XCO 2 ), is expected to become a key component of such an MVS capacity. Here we provide a novel assessment of the potential of a comprehensive data assimilation system using simulated XCO 2 and other observations to constrain fossil fuel CO 2 emission estimates for an exemplary 1-week period in 2008. We find that CO2M enables useful weekly estimates of country-scale fossil fuel emissions independent of national inventories. When extrapolated from the weekly to the annual scale, uncertainties in emissions are comparable to uncertainties in inventories, so that estimates from inventories and from the MVS capacity can be used for mutual verification. We further demonstrate an alternative, synergistic mode of operation, with the purpose of delivering a best fossil fuel emission estimate. In this mode, the assimilation system uses not only XCO 2 and the other data streams of the previous (verification) mode, but also the inventory information. Finally, we identify further steps towards an operational MVS capacity.
    Type of Medium: Online Resource
    ISSN: 1748-9326
    Language: Unknown
    Publisher: IOP Publishing
    Publication Date: 2022
    detail.hit.zdb_id: 2255379-4
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  • 4
    In: Atmospheric Science Letters, Wiley, Vol. 12, No. 1 ( 2011-01), p. 135-141
    Abstract: Real‐time surface and upper‐air observations are crucial to the analysis and forecasting of the West African monsoon (WAM). This paper will focus on the African Monsoon—Multidisciplinary Analyses (AMMA)‐driven reactivation and modernisation of the radiosonde network over West Africa, its potential long‐term impact on upper‐air operations in the region, the influence of the additional data in WAM analyses and forecasting, and the AMMA‐related development and usage of the West African Analysis/Forecasting (WASA/F) forecast method. Copyright © 2011 Royal Meteorological Society
    Type of Medium: Online Resource
    ISSN: 1530-261X , 1530-261X
    URL: Issue
    Language: English
    Publisher: Wiley
    Publication Date: 2011
    detail.hit.zdb_id: 2025884-7
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  • 5
    In: Remote Sensing, MDPI AG, Vol. 9, No. 10 ( 2017-10-16), p. 1052-
    Type of Medium: Online Resource
    ISSN: 2072-4292
    Language: English
    Publisher: MDPI AG
    Publication Date: 2017
    detail.hit.zdb_id: 2513863-7
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  • 6
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 21, No. 6 ( 2021-04-01), p. 5117-5136
    Abstract: Abstract. In this study, we present a novel monitoring methodology that combines satellite retrievals and forecasts to detect local CH4 concentration anomalies worldwide. These anomalies are caused by rapidly changing anthropogenic emissions that significantly contribute to the CH4 atmospheric budget and by biases in the satellite retrieval data. The method uses high-resolution (7 km × 7 km) retrievals of total column CH4 from the TROPOspheric Monitoring Instrument (TROPOMI) on board the Sentinel 5 Precursor satellite. Observations are combined with high-resolution CH4 forecasts (∼ 9 km) produced by the Copernicus Atmosphere Monitoring Service (CAMS) to provide departures (observations minus forecasts) at close to the satellite's native resolution at appropriate time. Investigating these departures is an effective way to link satellite measurements and emission inventory data in a quantitative manner. We perform filtering on the departures to remove the synoptic-scale and meso-alpha-scale biases in both forecasts and satellite observations. We then apply a simple classification scheme to the filtered departures to detect anomalies and plumes that are missing (e.g. pipeline or facility leaks), underreported or overreported (e.g. depleted drilling fields) in the CAMS emissions. The classification method also shows some limitations to detect emission anomalies only due to local satellite retrieval biases linked to albedo and scattering issues.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 7
    In: Atmospheric Measurement Techniques, Copernicus GmbH, Vol. 14, No. 2 ( 2021-02-26), p. 1525-1544
    Abstract: Abstract. The intensive measurement campaign CoMet 1.0 (Carbon Dioxide and Methane Mission) took place during May and June 2018, with a focus on greenhouse gases over Europe. CoMet 1.0 aimed at characterising the distribution of CH4 and CO2 over significant regional sources with the use of a fleet of research aircraft as well as validating remote sensing measurements from state-of-the-art instrumentation installed on board against a set of independent in situ observations. Here we present the results of over 55 h of accurate and precise in situ measurements of CO2, CH4 and CO mole fractions made during CoMet 1.0 flights with a cavity ring-down spectrometer aboard the German research aircraft HALO (High Altitude and LOng Range Research Aircraft), together with results from analyses of 96 discrete air samples collected aboard the same platform. A careful in-flight calibration strategy together with post-flight quality assessment made it possible to determine both the single-measurement precision as well as biases against respective World Meteorological Organization (WMO) scales. We compare the result of greenhouse gas observations against two of the available global modelling systems, namely Jena CarboScope and CAMS (Copernicus Atmosphere Monitoring Service). We find overall good agreement between the global models and the observed mole fractions in the free tropospheric range, characterised by very low bias values for the CAMS CH4 and the CarboScope CO2 products, with a mean free tropospheric offset of 0 (14) nmol mol−1 and 0.8 (1.3) µmol mol−1 respectively, with the numbers in parentheses giving the standard uncertainty in the final digits for the numerical value. Higher bias is observed for CAMS CO2 (equal to 3.7 (1.5) µmol mol−1), and for CO the model–observation mismatch is variable with height (with offset equal to −1.0 (8.8) nmol mol−1). We also present laboratory analyses of air samples collected throughout the flights, which include information on the isotopic composition of CH4, and we demonstrate the potential of simultaneously measuring δ13C−CH4 and δ2H−CH4 from air to determine the sources of enhanced methane signals using even a limited number of discrete samples. Using flasks collected during two flights over the Upper Silesian Coal Basin (USCB, southern Poland), one of the strongest methane-emitting regions in the European Union, we were able to use the Miller–Tans approach to derive the isotopic signature of the measured source, with values of δ2H equal to −224.7 (6.6) ‰ and δ13C to −50.9 (1.1) ‰, giving significantly lower δ2H values compared to previous studies in the area.
    Type of Medium: Online Resource
    ISSN: 1867-8548
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2505596-3
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  • 8
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 16, No. 3 ( 2016-02-12), p. 1653-1671
    Abstract: Abstract. This study presents results from the European Centre for Medium-Range Weather Forecasts (ECMWF) carbon dioxide (CO2) analysis system where the atmospheric CO2 is controlled through the assimilation of column-averaged dry-air mole fractions of CO2 (XCO2) from the Greenhouse gases Observing Satellite (GOSAT). The analysis is compared to a free-run simulation (without assimilation of XCO2), and they are both evaluated against XCO2 data from the Total Carbon Column Observing Network (TCCON). We show that the assimilation of the GOSAT XCO2 product from the Bremen Optimal Estimation Differential Optical Absorption Spectroscopy (BESD) algorithm during the year 2013 provides XCO2 fields with an improved mean absolute error of 0.6 parts per million (ppm) and an improved station-to-station bias deviation of 0.7  ppm compared to the free run (1.1 and 1.4  ppm, respectively) and an improved estimated precision of 1  ppm compared to the GOSAT BESD data (3.3  ppm). We also show that the analysis has skill for synoptic situations in the vicinity of frontal systems, where the GOSAT retrievals are sparse due to cloud contamination. We finally computed the 10-day forecast from each analysis at 00:00  UTC, and we demonstrate that the CO2 forecast shows synoptic skill for the largest-scale weather patterns (of the order of 1000  km) even up to day 5 compared to its own analysis.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2016
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 9
    In: Geoscientific Model Development, Copernicus GmbH, Vol. 10, No. 1 ( 2017-01-02), p. 1-18
    Abstract: Abstract. It is a widely established fact that standard semi-Lagrangian advection schemes are highly efficient numerical techniques for simulating the transport of atmospheric tracers. However, as they are not formally mass conserving, it is essential to use some method for restoring mass conservation in long time range forecasts. A common approach is to use global mass fixers. This is the case of the semi-Lagrangian advection scheme in the Integrated Forecasting System (IFS) model used by the Copernicus Atmosphere Monitoring Service (CAMS) at the European Centre for Medium-Range Weather Forecasts (ECMWF).Mass fixers are algorithms with substantial differences in complexity and sophistication but in general of low computational cost. This paper shows the positive impact mass fixers have on the inter-hemispheric gradient of total atmospheric column-averaged CO2 and CH4, a crucial feature of their spatial distribution. Two algorithms are compared: the simple "proportional" and the more complex Bermejo–Conde schemes. The former is widely used by several Earth system climate models as well the CAMS global forecasts and analysis of atmospheric composition, while the latter has been recently implemented in IFS. Comparisons against total column observations demonstrate that the proportional mass fixer is shown to be suitable for the low-resolution simulations, but for the high-resolution simulations the Bermejo–Conde scheme clearly gives better results. These results have potential repercussions for climate Earth system models using proportional mass fixers as their resolution increases. It also emphasises the importance of benchmarking the tracer mass fixers with the inter-hemispheric gradient of long-lived greenhouse gases using observations.
    Type of Medium: Online Resource
    ISSN: 1991-9603
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2017
    detail.hit.zdb_id: 2456725-5
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  • 10
    In: Earth System Science Data, Copernicus GmbH, Vol. 13, No. 11 ( 2021-11-17), p. 5311-5335
    Abstract: Abstract. The growth in anthropogenic carbon dioxide (CO2) emissions acts as a major climate change driver, which has widespread implications across society, influencing the scientific, political, and public sectors. For an increased understanding of the CO2 emission sources, patterns, and trends, a link between the emission inventories and observed CO2 concentrations is best established via Earth system modelling and data assimilation. Bringing together the different pieces of the puzzle of a very different nature (measurements, reported statistics, and models), it is of utmost importance to know their level of confidence and boundaries well. Inversions disaggregate the variation in observed atmospheric CO2 concentration to variability in CO2 emissions by constraining the regional distribution of CO2 fluxes, derived either bottom-up from statistics or top-down from observations. The level of confidence and boundaries for each of these CO2 fluxes is as important as their intensity, though often not available for bottom-up anthropogenic CO2 emissions. This study provides a postprocessing tool CHE_UNC_APP for anthropogenic CO2 emissions to help assess and manage the uncertainty in the different emitting sectors. The postprocessor is available under https://doi.org/10.5281/zenodo.5196190 (Choulga et al., 2021). Recommendations are given for regrouping the sectoral emissions, taking into account their uncertainty instead of their statistical origin; for addressing local hot spots; for the treatment of sectors with small budget but uncertainties larger than 100 %; and for the assumptions around the classification of countries based on the quality of their statistical infrastructure. This tool has been applied to the EDGARv4.3.2_FT2015 dataset, resulting in seven input grid maps with upper- and lower-half ranges of uncertainty for the European Centre for Medium-Range Weather Forecasts Integrated Forecasting System. The dataset is documented and available under https://doi.org/10.5281/zenodo.3967439 (Choulga et al., 2020). While the uncertainty in most emission groups remains relatively small (5 %–20 %), the largest contribution (usually over 40 %) to the total uncertainty is determined by the OTHER group (of fuel exploitation and transformation but also agricultural soils and solvents) at the global scale. The uncertainties have been compared for selected countries to those reported in the inventories submitted to the United Nations Framework Convention on Climate Change and to those assessed for the European emission grid maps of the Netherlands Organisation for Applied Scientific Research. Several sensitivity experiments are performed to check (1) the country dependence (by analysing the impact of assuming either a well- or less well-developed statistical infrastructure), (2) the fuel type dependence (by adding explicit information for each fuel type used per activity from the Intergovernmental Panel on Climate Change), and (3) the spatial source distribution dependence (by aggregating all emission sources and comparing the effect against an even redistribution over the country). The first experiment shows that the SETTLEMENTS group (of energy for buildings) uncertainty changes the most when development level is changed. The second experiment shows that fuel-specific information reduces uncertainty in emissions only when a country uses several different fuels in the same amount; when a country mainly uses the most globally typical fuel for an activity, uncertainty values computed with and without detailed fuel information are the same. The third experiment highlights the importance of spatial mapping.
    Type of Medium: Online Resource
    ISSN: 1866-3516
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2475469-9
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