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  • 1
    Online Resource
    Online Resource
    New York, NY : Springer Science+Business Media, LLC
    UID:
    b3kat_BV036650337
    Format: 1 Online-Ressource , v.: digital
    Edition: Online_Ausgabe New York, NY Springer Science+Business Media, LLC 2006 Springer ebook collection / Chemistry and Materials Science 2005-2008 Sonstige Standardnummer des Gesamttitels: 041171-1
    ISBN: 9780387284293 , 9780387284309
    Additional Edition: Reproduktion von N4-Macrocyclic Metal Complexes 2006
    Language: English
    URL: Cover
    URL: Volltext  (lizenzpflichtig)
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  • 2
    Online Resource
    Online Resource
    New York :Springer,
    UID:
    edocfu_9958073703602883
    Format: 1 online resource (831 p.)
    Edition: 1st ed. 2006.
    ISBN: 1-280-72409-9 , 9786610724093 , 0-387-28430-3
    Content: Offers insight into the various applications and developments of N4 macrocycle complexes in the field of biomimetic electrocatalysis. This book is devoted to the chemistry, electronic and electrochemical properties of porphyrin-based polymetallated supramolecular redox catalysts and their applications in photoelectrochemical molecular devices.
    Note: Description based upon print version of record. , Billion-Year-Old Oxygen Cathode that Actually Works: Respiratory Oxygen Reduction and Its Biomimetic Analogs -- Fundamental Aspects on the Catalytic Activity of Metallomacrocyclics for the Electrochemical Reduction of O2 -- Oxygen Reduction in PEM Fuel Cell Conditions: Heat-Treated Non-Precious Metal-N4 Macrocycles and Beyond -- Biomimetic NOx Reductions by Heme Models and Proteins -- Electroreduction of CO2 Catalyzed by Metallomacrocyclics -- Supramolecular Porphyrins as Electrocatalysts -- Electrodes Modified with Monomeric M-N4 Catalysts for the Detection of Environmentally Important Molecules -- Electropolymerized Metalloporphyrin Metallophthalocyanine and Metal Schiff Base Complex Films: Applications to Biomimetic Electrocatalysis and Bioelectroanalysis -- Electron Transfer Processes of ?-Pyrrole Brominated Porphyrins: Structural vs. Electronic Effects -- Photoelectrochemical Reactions at Phthalocyanine Electrodes -- Organisation and Photoelectrochemical Reactivity of Water-Soluble Metalloporphyrins at the Liquid/Liquid Interface -- Theoretical Insights on the Chemical Reactivity of Metalloporphyrins Using Density Functional Theory -- Organized Multiporphyrinic Assemblies for Photoconduction and Electroconduction -- Vibrational Spectra and Surface-Enhanced Vibrational Spectra of Azamacrocycles. , English
    Additional Edition: ISBN 0-387-28429-X
    Language: English
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  • 3
    UID:
    almafu_9959328222702883
    Format: 1 online resource (xviii, 428 pages)
    ISBN: 9783527664900 , 9783527664931 , 3527664939 , 3527664904 , 9781306550482 , 1306550483
    Content: Written and edited by top fuel cell catalyst scientists and engineers from both industry and academia, this is the first book to provide a complete overview of this hot topic. It covers the synthesis, characterization, activity validation and modeling of different non-noble metal electrocatalysts, as well as their integration into fuel cells and their performance validation, while also discussing those factors that will drive fuel cell commercialization. With its well-structured approach, this is a must-have for researchers working on the topic, and an equally valuable companion for newcomers to the field.
    Note: Non-Noble Metal Fuel Cell Catalysts; Contents; Preface; List of Contributors; Chapter 1 Electrocatalysts for Acid Proton Exchange Membrane (PEM) Fuel Cells -- an Overview; 1.1 Introduction; 1.2 Acid PEM Fuel Cell Background and Fundamentals; 1.2.1 Acid PEM Fuel Cell Overview -- History, Status, and Advantages; 1.2.2 Acid PEM Fuel Cell Reactions -- Thermodynamics and Kinetics; 1.3 Acid PEM Fuel Cell Catalysis for Cathode O2 Reduction Reaction; 1.3.1 Electrochemical Thermodynamics of O2 Reduction Reaction; 1.3.2 Pt-Based Catalysts for the Oxygen Reduction Reaction. , 1.3.3 Electrochemical Kinetics and Mechanism of the O2 Reduction Reaction Catalyzed by Pt Catalysts1.4 Catalyst Challenges and Perspective in Acid PEM Fuel Cells; 1.4.1 Pt Catalyst Cost Analysis and Major Challenges; 1.4.2 Sustainability; 1.4.3 Major Technical Challenges for Non-noble Metal Catalysts and Mitigation Strategies; 1.4.4 Non-noble Metal Catalyst Overview; 1.5 Conclusion; References; Chapter 2 Heat-Treated Transition Metal-NxCy Electrocatalysts for the O2 Reduction Reaction in Acid PEM Fuel Cells; 2.1 Introduction. , 2.1.1 Why the Search for Non-precious Metal Catalysts for O2 Reduction?2.1.2 Activity, Power Performance, and Durability Constraints on Me/N/C Catalysts; 2.1.3 Milestones Achieved by Me/N/C Catalysts over the Last 50 Years; 2.1.3.1 Milestone 1; 2.1.3.2 Milestone 2; 2.1.3.3 Milestone 3; 2.1.3.4 Milestone 4; 2.1.3.5 Milestone 5; 2.2 Synthesis Approaches for Heat-Treated Me/N/C Catalysts; 2.2.1 The Supported-Macrocycle Approach; 2.2.2 The Templating Method; 2.2.3 The Foaming Agent Approach; 2.2.4 The N Molecule or Metal-Ligand Approach; 2.2.5 The N-Polymer Approach. , 2.2.6 Gaseous N-Precursor Approach (NH3 and CH3CN)2.2.7 Thermally Decomposable Metal-Organic Frameworks (MOF); 2.3 Important Parameters for Highly Active Me/N/C Catalysts; 2.3.1 Pyrolysis Temperature; 2.3.1.1 Metal Macrocycles Supported on Carbon and Pyrolyzed in Inert Atmosphere; 2.3.1.2 Separate Metal and Nitrogen Precursors or Metal-Ligand Complexes Impregnated on a Carbon Support and Pyrolyzed in Inert or Reactive Atmosphere; 2.3.2 The Transition Metal; 2.3.2.1 Binary Metal Catalysts; 2.3.2.2 Metal Concentration. , 2.3.3 The Nitrogen Content and Speciation by X-ray Photoelectron Spectroscopy (XPS)2.3.4 The Carbon Support/Host; 2.4 Nature of the Active Sites; 2.4.1 Time-of-Flight Secondary Ion Mass Spectroscopy; 2.4.2 X-ray Absorption Spectroscopy and Extended X-ray Absorption Fine Structure; 2.4.2.1 Studies on Pyrolyzed Macrocycles; 2.4.2.2 Studies on Catalysts Synthesized from Separate Metal, N and C Precursors; 2.4.3 Mössbauer Spectroscopy; 2.4.3.1 Studies on FePc and Fe- Porphyrin, Unpyrolyzed or Pyrolyzed at T 〈500 °C; 2.4.3.2 Studies on Fe Macrocycles Pyrolyzed at T e"700 °C.
    Additional Edition: Print version: Non-noble metal fuel cell catalysts. Weinheim, Germany : Wiley-VCH, [2014] ISBN 9783527333240
    Language: English
    Keywords: Electronic books. ; Electronic books. ; Electronic books. ; Electronic books. ; Electronic books. ; Electronic books.
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