Format:
1 Online-Ressource (8 Seiten)
ISSN:
1438-1656
,
1527-2648
,
1438-1656
,
1527-2648
Content:
Thin-film perovskite light-emitting diodes have gained increasing attention in the last 6 years. With the possibility to process the emitting layer from solution, the way for 1D morphology of the semiconductor for flexible devices is paved. Herein, for the first time single-step fabrication of CsPbBr3@PVP nanofibers in a customized electrospinning process performed under ambient conditions from a water-based precursor solution is reported. The water-based approach allows the incorporation of a conductive polymer into the compound fiber by blending the perovskite precursor ink with commercially available PEDOT:PSS dispersion. The results demonstrate electrospun fiber mats which are stable at ambient conditions for at least 5 months and can be utilized in electroluminescence devices. Photoluminescence studies on the perovskite fibers reveal a blueshift of the emission peak compared to thin films possibly due to the generation of nanocrystals of ≈12 nm by in situ nanocrystal pinning as confirmed by transmission electron microscopy. A proof-of-concept electrically pumped light-emitting device is built with the obtained fiber mat. The perovskite nanofibers offer promising applications in flexible and stretchable optoelectronics.
Content:
Peer Reviewed
In:
Weinheim : Wiley-VCH, 25,10, 1438-1656
In:
1527-2648
Language:
English
DOI:
10.1002/adem.202201651
URN:
urn:nbn:de:kobv:11-110-18452/27838-8
URL:
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