Format:
1 Online-Ressource (12 Seiten)
Content:
Recent advances in coherent multidimensional spectroscopy have boosted interest in exciton coherences in light harvesting complexes. We present nonperturbative calculations of two-dimensional (2D) electronic spectroscopy from a fifth-order phase-matching direction. The calculations show clear patterns that correspond to the electronic structure of one- and two-exciton manifolds of a Fenna–Matthews–Olsson light harvesting complex. Such signals can provide new information about the coherent properties of antenna pigment protein complexes.
Content:
Peer Reviewed
In:
[London] : IOP, 13,2
Language:
English
DOI:
10.1088/1367-2630/13/2/025024
URN:
urn:nbn:de:kobv:11-110-18452/25901-7
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