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  • BSZ  (5)
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  • 1
    Online Resource
    Online Resource
    Cham : Springer International Publishing
    UID:
    (DE-627)1030109184
    Format: Online-Ressource (XXI, 117 p. 46 illus. in color, online resource)
    Edition: Springer eBook Collection. Physics and Astronomy
    ISBN: 9783319982526
    Series Statement: Springer Theses, Recognizing Outstanding Ph.D. Research
    Content: This book focuses on the characterisation of the chiral and topological nature of magnetic skyrmions in noncentrosymmetric helimagnets. In these materials, the skyrmion lattice phase appears as a long-range-ordered, close-packed grid of nearly millimetre-level correlation length, while the size of a single skyrmion is 3-100 nm. This is a very challenging range of length scales (spanning 5 orders of magnitude from tens of nm to mm) for magnetic characterisation techniques, and, to date, extensive information on this fascinating, magnetically ordered state has remained elusive. In response, this work develops novel resonant elastic x-ray scattering (REXS) techniques, which allow the magnetic structure, including the long-range order and domain formation, as well as microscopic skyrmion parameters, to be measured across the full range of length scales. Most importantly, using circular dichroism in REXS, the internal structure of a given skyrmion, the topological winding number, and the skyrmion helicity angle can all be unambiguously determined. These new techniques are applicable to many materials systems, and allow us to retrieve information on modulated spin structures, multiferroic order, spin-density-waves, and other forms of topological magnetic order
    Content: The Story so Far -- Measurement of the Magnetic Long-range Order -- Measurement of the Skyrmion Lattice Domains -- Measurement of the Topological Winding Number -- Measurement of the Skyrmion Helicity Angle -- Dichroism Extinction Rule
    Additional Edition: 9783319982519
    Additional Edition: 9783319982533
    Additional Edition: Erscheint auch als Druck-Ausgabe 978-3-319-98251-9
    Additional Edition: Printed edition 9783319982519
    Additional Edition: Printed edition 9783319982533
    Language: English
    Keywords: Magnetisches Skyrmion ; Spintronik ; Chirale Symmetrie ; Topologische Phase ; Röntgenstreuung ; Dichroismus ; Extinktion
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  • 2
    Online Resource
    Online Resource
    Cham : Springer
    UID:
    (DE-627)1688302999
    Format: 1 online resource (134 pages)
    ISBN: 9783319982526
    Series Statement: Springer Theses Ser.
    Content: Intro -- Supervisor's Foreword -- Abstract -- Parts of this thesis have been published in the following journal articles:Chapter 1: S. Zhang, A. A. Baker, S. Komineas, and T. Hesjedal, "Topological computation based on direct magnetic logic communication", Sci. Rep. 5, 1773 (2015).Chapter 2: A. I. Figueroa, S. L. Zhang, A. A. Baker, R. Chalasani, A. Kohn, S. C. Speller, D. Gianolio, C. Pfleiderer, G. van der Laan, and T. Hesjedal, "Strain in epitaxial MnSi films on Si(111) in the thick film limit studied by polarization-dependent extended x -- Acknowledgements -- Contents -- Acronyms -- 1 The Story So Far -- 1.1 Theoretical Treatments -- 1.1.1 Skyrme Field in the Non-linear Sigma Model -- 1.1.2 The Theory of Magnetic Skyrmions -- 1.1.3 Magnetism of P213 Helimagnets -- 1.2 The Properties of Magnetic Skyrmions -- 1.2.1 Interaction with Conduction Electrons -- 1.2.2 Interaction with Magnons -- 1.3 Characterisation of Magnetic Skyrmions -- 1.3.1 Magnetic Neutron Diffraction -- 1.3.2 Lorentz Transmission Electron Microscopy -- 1.3.3 Magnetic Force Microscopy -- 1.4 What Is Missing? -- 1.5 Structure of the Thesis -- References -- 2 Measurement of the Magnetic Long-Range Order -- 2.1 Writing Down the Scattering Process -- 2.1.1 Scattering from a Single Electron -- 2.1.2 Scattering from a Single Atom -- 2.1.3 Scattering from a Periodic Lattice -- 2.1.4 Scattering from Helical, Conical, and Skyrmion Order -- 2.2 REXS in Reflection Geometry -- 2.2.1 Results -- 2.3 REXS in Grazing Geometry -- References -- 3 Measurement of the Skyrmion Lattice Domains -- 3.1 Diffraction from the Multidomain Skyrmion Lattice State -- 3.2 Imaging of the Multidomain Skyrmion Lattice State -- 3.3 Domain Boundary Structure -- References -- 4 Measurement of the Topological Winding Number -- 4.1 REXS Polarisation Dependence -- 4.2 Topology Determination Principle.
    Note: Description based on publisher supplied metadata and other sources
    Additional Edition: 9783319982519
    Additional Edition: Erscheint auch als Druck-Ausgabe 9783319982519
    Language: English
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  • 3
    UID:
    (DE-627)1811875521
    ISSN: 2666-3864
    Content: Rechargeable Na-CO2 batteries are promising energy-storage devices due to their high energy density, environmental friendliness, and cost effectiveness. However, the insulating nature and irreversibility of the Na2CO3 discharge product cause large polarization and poor cyclicity. Here, we report a reversible quasi-solid-state Na-CO2 battery that is constructed by the synergistic action of a Co-encapsulated N-doped carbon framework catalyst and gel electrolyte to ensure the formation of a highly reversible Na2C2O4 discharge product. Experiments and density functional theory calculations indicate that the electron-agglomeration effect of Co nanoparticles enhances CO2 adsorption and lowers energy barrier, as well as promotes Na2C2O4 generation. A gel electrolyte containing an imidazole organic cation is used to inhibit the decomposition of the thermodynamically unstable Na2C2O4. The fabricated Na-CO2 battery exhibits a high discharge capacity of 3,094 mAh g^-1, a high-rate performance of 1,777 mAh g^-1 at a current density of 0.5 mA cm^-2, and excellent cycling performance of 366 cycles (2,200 h).
    In: Cell reports. Physical science, Maryland Heights, MO : Cell Press, 2020, 3(2022), 7, Artikel-ID 100973, Seite 1-15, 2666-3864
    In: volume:3
    In: year:2022
    In: number:7
    In: elocationid:100973
    In: pages:1-15
    Language: English
    URL: Volltext  (kostenfrei)
    URL: Volltext  (kostenfrei)
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  • 4
    UID:
    (DE-627)1810403308
    Format: 1 Online-Ressource (26 p)
    Content: We developed a [001] B2 preferentially oriented Co-Ni-Ga alloy with Cu and B co-alloying, which contains two kinds of ductile secondary phases precipitated in the columnar grain interior and grain boundaries, respectively. This textured Co-Ni-Ga-Cu-B heterostructural alloy presents remarkable mechanical behaviors with a high yield strength of ~1300 MPa and an appreciable failure strain of ~8.8%. An exceptional superelasticity combined with fully reversible strain of 2.5%, low driving force of 99 MPa, narrow stress hysteresis of 33.5 MPa and extraordinary mechanical cyclic stability for 20,000 cycles was also successfully achieved in the studied alloy. By virtue of its superior mechanical responses, an excellent room-temperature elastocaloric effect showing a moderate adiabatic temperature change of -3.2 K at a small transformation strain of 1.5% was observed over 20,000 cycles without any apparent degradation. More importantly, the fatigue resistance of superelasticity and elastocaloric effect is extremely enhanced relative to the reported single-crystal counterparts. The great performances of superelasticity and elastocaloric effect of the optimized Co-Ni-Ga alloy imply a promising future for advanced superelastic and solid-state refrigeration applications, and the collaborative design approach may be exploited to other intermetallic-type shape memory alloys
    Language: English
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  • 5
    UID:
    (DE-627)1688121331
    ISSN: 2041-1723
    In: Nature Communications, [London] : Nature Publishing Group UK, 2010, 11(2020) vom: 15. Jan., Artikel-ID 299, Seite 1-10, 2041-1723
    In: volume:11
    In: year:2020
    In: day:15
    In: month:01
    In: elocationid:299
    In: pages:1-10
    Language: English
    URL: Volltext  (kostenfrei)
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