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Toward physical aspects affecting a possible leakage of geologically stored CO2 into the shallow subsurface

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Abstract

In geological formations, migration of CO2 plume is very complex and irregular. To make CO2 capture and storage technology feasible, it is important to quantify CO2 amount associated with possible leakage through natural occurring faults and fractures in geologic medium. Present work examines the fracture aperture effect on CO2 migration due to free convection. Numerical results reveal that fracture with larger-aperture intensify CO2 leakage. Mathematical formulation and equations of state for the mixture are implemented within the object-oriented finite element code OpenGeoSys developed by the authors. The volume translated Peng–Robinson equation of state is used for material properties of CO2 and water.

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References

  1. Ahlers J, Gmehling J (2001) Development of a universal group contribution equation of state: prediction of liquid densities for pure compounds with a volume translated Peng-Robinson equation of state. Fluid Phase Equilib 191:177–188

    Article  Google Scholar 

  2. Bear J (1972) Dynamics of fluid in porous media. Elsevier, New York

    Google Scholar 

  3. Diersch H-JG, Kolditz O (2002) Variable-density flow and transport in porous media: approaches and challenges. Adv Water Resour 25:899–944

    Article  Google Scholar 

  4. Elder JW (1967) Transient convection in a porous medium. J Fluid Mech 27:609–623

    Article  Google Scholar 

  5. Kolditz O, Bauer S, Bilke L, Böttcher N, Delfs JO, Fischer T, Görke UJ, Kalbacher T, Kosakowski G, McDermott CI, Park CH, Radu F, Rink K, Shao H, Shao HB, Sun F, Sun YY, Singh AK, Taron J, Walther M, Wang W, Watanabe N, Wu N, Xie M, Xu W, Zehner B (2012) OpenGeoSys: an open source initiative for numerical simulation of thermo-hydro-mechanical/chemical (THM/C) processes in porous media. Environ Earth Sci 67(2):589–599

    Article  Google Scholar 

  6. Kolditz O, Shao H, Wang W (2012) Benchmarks and examples for thermo-hydro mechanical/chemical processes in porous media, 1st edn. Springer, Berlin

    Book  Google Scholar 

  7. Murphy HD (1979) Convective instabilities in vertical fractures and faults. J Geophy Res 84:6121–6130

    Article  Google Scholar 

  8. Pan L, Oldenburg CN, Wu Y, Pruess K (2009) Wellbore flow model for carbon dioxide and brine. Energy Procedia 1:71–78

    Article  Google Scholar 

  9. Peng DY, Robinson DB (1976) A new two-constant equation of state. Ind Eng Chem Fundam 15:59–64

    Article  MATH  Google Scholar 

  10. Prasad A, Simmons CT (2003) Unstable density-driven flow in heterogeneous porous media: a stochastic study of the Elder [1967b] “short heater” problem. Water Resour Res 39:1007. doi:10.1029/2002WR001290

    Article  Google Scholar 

  11. Singh AK, Böettcher N, Wang W, Park C-H, Görke U-J, Kolditz O (2011) Non-isothermal effects on two-phase flow in porous medium: CO2 disposal into a saline aquifer. Energy Procedia 4:3889–3895

    Article  Google Scholar 

  12. Shi M (2005) Characterizing heterogeneity in low-permeability strata and its control on fluid flow and solute transport by thermohaline free convection. Unpublished Ph.D. thesis, University of Texas at Austin 229 pp

  13. Shikaze SG, Sudicky EA, Schwartz FW (1998) Density-dependent solute transport in discretely-fractured geologic media: is prediction possible? J Contamin Hydrol 34:273–291

    Article  Google Scholar 

  14. Tsai J-C, Chen Y-P (1998) Application of a volume translated Peng-Robinson equation of state on vapore liquid equilibrium calculations. Fluid Phase Equilib 145:193–215

    Article  Google Scholar 

  15. Taylor GI (1954) Diffusion and mass transport in tubes. Proc Phys Soc B 67 (12):857–869

    Google Scholar 

  16. Wooding RA (1957) Steady state free thermal convection of liquid in a saturated permeable medium. J Fluid Mech 2:273–285

    Article  MATH  MathSciNet  Google Scholar 

Download references

Acknowledgments

We acknowledge the funding by the German Federal Ministry of Education and Research (BMBF) within the framework of the CO2BENCH (FKZ 03G0797D) project as a part of the Special Program GEOTECHNOLOGIEN.

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Correspondence to Ashok Singh.

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Singh, A., Delfs, J.O., Görke, U.J. et al. Toward physical aspects affecting a possible leakage of geologically stored CO2 into the shallow subsurface. Acta Geotech. 9, 81–86 (2014). https://doi.org/10.1007/s11440-013-0237-4

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  • DOI: https://doi.org/10.1007/s11440-013-0237-4

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